Free-Space–Coupled Frequency-Locked Microtoroid Resonators for Ultrasensitive Gas-Phase Detection

Happy to share our latest paper in Laser & Photonics Reviews.
We demonstrate free-space–coupled, frequency-locked microtoroid resonators for gas sensing—overcoming the long-standing limitation of fragile fiber tapers and moving WGM sensors closer to real-world use.
We accomplished:
• 25 ppt detection limit at room temperature
• >10⁷ Q factors preserved after polymer coating
• 3 orders of magnitude improvement over prior work
• Compact, robust, and capable of long-duration, unattended sensing
Using a mustard gas simulant (2-CEES), we show that ultrahigh sensitivity and real-world robustness can coexist.
This is the first demonstration of free-space–coupled WGM microtoroids for chemical sensing, opening new opportunities in defense, security, and environmental monitoring.
Thanks to our excellent collaborators and generous sponsors.

Free‐Space‐Coupled Frequency‐Locked Microtoroid Resonators With Reactive Polymer Functionalization for Part‐Per‐Trillion Gas Detection – Xu – Laser & Photonics Reviews – Wiley Online Library